2020
DOI: 10.1103/physrevresearch.2.023070
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Rearrangement of two dimensional aggregates of droplets under compression: Signatures of the energy landscape from crystal to glass

Abstract: We study signatures of the energy landscape's evolution through the crystal-to-glass transition by compressing two dimensional (2D) finite aggregates of oil droplets. Droplets of two distinct sizes are used to compose small aggregates in an aqueous environment. Aggregates range from perfectly ordered monodisperse single crystals to disordered bidisperse glasses. The aggregates are compressed between two parallel boundaries, with one acting as a force sensor. The compression force provides a signature of the ag… Show more

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Cited by 10 publications
(7 citation statements)
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“…Using bubbles instead of atoms, dislocations and grain boundaries were imaged directly and mechanical properties of the assembly were studied 2 . The use of foams, emulsions, and colloids has become a powerful tool to study fundamental questions such as the glass transition [3][4][5][6][7][8] , formation and melting of crystals [9][10][11][12] , the order-to-disorder transition [13][14][15][16][17][18] and jamming [19][20][21][22][23][24] . Complex biological systems can also be modeled using foams and emulsions [25][26][27][28] .…”
Section: Introductionmentioning
confidence: 99%
“…Using bubbles instead of atoms, dislocations and grain boundaries were imaged directly and mechanical properties of the assembly were studied 2 . The use of foams, emulsions, and colloids has become a powerful tool to study fundamental questions such as the glass transition [3][4][5][6][7][8] , formation and melting of crystals [9][10][11][12] , the order-to-disorder transition [13][14][15][16][17][18] and jamming [19][20][21][22][23][24] . Complex biological systems can also be modeled using foams and emulsions [25][26][27][28] .…”
Section: Introductionmentioning
confidence: 99%
“…Micropipette force sensor measurements. Micropipette force sensors have recently been extensively used in various biophysical [30][31][32][33][34][35][36][37][38][39] and soft matter 40,41 studies (see ref. 42 for a complete review and protocol and ref.…”
Section: Resultsmentioning
confidence: 99%
“…The keyword here is "optimal", and it concerns the deterministic and random packing of inclusions in R d . Studies of packing advance our knowledge about the effective properties of densely packed composites, porous and granular media, metallic glasses, and emulsions [1][2][3].…”
Section: Introductionmentioning
confidence: 99%
“…The spatially symmetric arrays of disks, i.e., the hexagonal (triangular) lattice in R 2 and the FCC or HCP lattice in R 3 , naturally arise in a deterministic statement. Random optimal packing is usually related to random-walk algorithms and their implementation (see [1][2][3][4] and references therein). In the present paper, we develop the theory of optimal random packing.…”
Section: Introductionmentioning
confidence: 99%