“…Understanding the efficiency of sympathetic cooling is critical in fields such as quantum information processing, where cooling the computational ions has been described as the “runtime bottleneck” . While sympathetic cooling has been experimentally measured in very small crystals (with <5 ions), ,, it is challenging to apply these techniques to more complex systems, and sympathetic cooling in larger crystals has been predominantly studied using detailed simulations. − The time-dependent kinetic energy distribution of laser-irradiated 113 Cd + ions was recently experimentally measured in large bicomponent Cd + –Ca + Coulomb crystals . However, as this approach was based on the Doppler broadening of the 113 Cd + fluorescence signal, it cannot be straightforwardly applied to the majority of (nonfluorescing) cotrapped species that are of interest in ion reactivity studies.…”