Articles you may be interested inTiO2@Silica nanoparticles in a random laser: Strong relationship of silica shell thickness on scattering medium properties and random laser performance Appl. Phys. Lett. 104, 081909 (2014); 10.1063/1.4865092SiO 2 nanoparticles as scatterers for random organic laser action in red fluorescent dye 4-(dicyanomethylene)-2tert-butyl-6(1,1,7,7-tetramethyljulolidyl-9-enyl)-4 H -pyran doped polystyrene films Random lasing emission from a red fluorescent dye doped polystyrene film containing dispersed polystyrene nanoparticles Appl. Phys. Lett. 91, 091115 (2007);We studied the random laser (RL) bichromatic emission (BCE) from a powder consisting of silica particles infiltrated with Rhodamine 640 (Rh640) molecules. The BCE is attributed to Rh640 monomers and dimers. Because of the efficient monomer-dimer energy transfer, we observed RL wavelength switching from % 620 nm to %650 nm and the control of the emitted wavelength was made by changing only the excitation laser intensity. None of external parameters such as excitation laser spot size or radiation detector position was changed as in previous experiments. Two laser thresholds associated either to monomers or dimers were clearly observed. Moreover, an effect analog to frequency-pulling among two coupled oscillators was identified measuring the RL spectra as a function of the excitation laser intensity. A wavelength shift, Dk, was measured between the monomer and dimer resonance wavelengths, changing only the excitation laser intensity. The maximum value of Dk % 16 cm À1 was obtained for laser pulses of 7 ns with 30 lJ. V C 2014 AIP Publishing LLC. [http://dx.doi.org/10.1063/1.4863308]
043515-3Barbosa-Silva et al.