Abstract:We introduce the quantum stochastic walk (QSW), which determines the evolution of generalized quantum mechanical walk on a graph that obeys a quantum stochastic equation of motion. Using an axiomatic approach, we specify the rules for all possible quantum, classical and quantum-stochastic transitions from a vertex as defined by its connectivity. We show how the family of possible QSWs encompasses both the classical random walk (CRW) and the quantum walk (QW) as special cases, but also includes more general pro… Show more
“…Nevertheless there are many other mechanism of decoherence, see for example [31]. To our knowledge this pioneer problem was well posed in van Kampen's paper [12], but many other related approaches have also been presented in the literature [15,40]. The propagation of photons in waveguide lattices have been studied in recent years [24,25], and they are possible scenarios where our present results can be applied.…”
We have investigated the time-evolution of a free particle in interaction with a phonon thermal bath, using the tight-binding approach. A dissipative quantum walk can be defined and many important non-equilibrium decoherence properties can be investigated analytically. The non-equilibrium statistics of a pure initial state have been studied. Our theoretical results indicate that the evolving wave-packet shows the suppression of Anderson's boundaries (ballistic peaks) by the presence of dissipation. Many important relaxation properties can be studied quantitatively, such as von Neumann's entropy and quantum purity. In addition, we have studied Wigner's function. The time-dependent behavior of the quantum entanglement between a free particle -in the lattice-and the phonon bath has been characterized analytically. This result strongly suggests the non-trivial time-dependence of the off-diagonal elements of the reduced density matrix of the system. We have established a connection between the quantum decoherence and the dissipative parameter arising from interaction with the phonon bath. The time-dependent behavior of quantum correlations has also been pointed out, showing continuous transition from quantum random walk to classical random walk, when dissipation increases.
“…Nevertheless there are many other mechanism of decoherence, see for example [31]. To our knowledge this pioneer problem was well posed in van Kampen's paper [12], but many other related approaches have also been presented in the literature [15,40]. The propagation of photons in waveguide lattices have been studied in recent years [24,25], and they are possible scenarios where our present results can be applied.…”
We have investigated the time-evolution of a free particle in interaction with a phonon thermal bath, using the tight-binding approach. A dissipative quantum walk can be defined and many important non-equilibrium decoherence properties can be investigated analytically. The non-equilibrium statistics of a pure initial state have been studied. Our theoretical results indicate that the evolving wave-packet shows the suppression of Anderson's boundaries (ballistic peaks) by the presence of dissipation. Many important relaxation properties can be studied quantitatively, such as von Neumann's entropy and quantum purity. In addition, we have studied Wigner's function. The time-dependent behavior of the quantum entanglement between a free particle -in the lattice-and the phonon bath has been characterized analytically. This result strongly suggests the non-trivial time-dependence of the off-diagonal elements of the reduced density matrix of the system. We have established a connection between the quantum decoherence and the dissipative parameter arising from interaction with the phonon bath. The time-dependent behavior of quantum correlations has also been pointed out, showing continuous transition from quantum random walk to classical random walk, when dissipation increases.
“…If only the coherent term was present the QSW would correspond to a standard CTQW. On the other hand, it can be shown that if only the incoherent term was present the QSW would correspond to a classical random walk for the diagonal elements of ρ(t) [22]. A standard stochastic method to study the dynamics described by eq.…”
Section: Quantum Stochastic Walksmentioning
confidence: 99%
“…QSWs are a class of stochastic processes introduced in [22] with the purpose of generalizing both continuous time quantum walks, and classical random walks [29] into a single framework. A QSW is specified by a quantum master equation in Lindblad form [30] describing the evolution of the system's density matriẋ…”
Section: Quantum Stochastic Walksmentioning
confidence: 99%
“…The rest of the paper is divided as follows: in the second section we define the notion of QSW as introduced in [22]; in the third section we provide a brief introduction to the LD approach; in the fourth section we apply the thermodynamic formalism to describe the dynamics of a QSW on a directed graphs; while the last section is devoted to discussions and conclusions.…”
Section: Introductionmentioning
confidence: 99%
“…In this work, following [22], we will refer to dissipative CTQWs as Quantum Stochastic Walks (QSWs). Using the quantum jump approach [23] we study the statistical properties of the ensemble of trajectories originated by QSWs.…”
We consider the dynamical properties of dissipative continuous time quantum walks on directed graphs. Using a large deviation approach we construct a thermodynamic formalism allowing us to define a dynamical order parameter, and to identify transitions between dynamical regimes. For a particular class of dissipative quantum walks we propose a new quantum generalization of the the classical pagerank vector, used to rank the importance of nodes in a directed graph. We also provide an example where one can characterize the dynamical transition from an effective classical random walk to a dissipative quantum walk as a thermodynamic crossover between distinct dynamical regimes.
The implementation of probabilistic algorithms by deterministic hardware is demanding and requires hundreds of instructions to generate a pseudo-random sequence of numbers. On the contrary, the dynamics at the molecular scale is physically governed by probabilistic laws because of the stochastic nature of thermally activated and quantum processes. By simulating the exciton transfer dynamics in a multi-chromophoric system, we demonstrate the implementation of a random walk that samples the possible pathways of a traveler through a network and can be probed by time-resolved fluorescence spectroscopy. The ability of controlling the spatial arrangement of the chromophores allows us to design the "landscape" in which the traveler is moving and therefore to program the molecular device
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