2014
DOI: 10.1103/physrevlett.112.046601
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Quantum Nature of Edge Magnetism in Graphene

Abstract: It is argued that the subtle crossover from decoherence-dominated classical magnetism to fluctuation-dominated quantum magnetism is experimentally accessible in graphene nanoribbons. We show that the width of a nanoribbon determines whether the edge magnetism is on the classical side, on the quantum side, or in between. In the classical regime, decoherence is dominant and leads to static spin polarizations at the ribbon edges, which are well described by mean-field theories. The quantum Zeno effect is identifi… Show more

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Cited by 67 publications
(71 citation statements)
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“…It is known that the ground state for the Heisenberg model on a finite bipartite lattice is a spin singlet. According to the DMRG calculations, we find that the ground state30 is very close to the Néel state. Figure 4 shows the magnetization profiles 〈 S z ( r )〉 in the lowest-energy state of ∑ r S z ( r ) = 0 for the Heisenberg model with a local Zeeman field − hS z ( r 0 ) applied to the center site r 0 at the upper edge.…”
Section: Discussionmentioning
confidence: 68%
See 1 more Smart Citation
“…It is known that the ground state for the Heisenberg model on a finite bipartite lattice is a spin singlet. According to the DMRG calculations, we find that the ground state30 is very close to the Néel state. Figure 4 shows the magnetization profiles 〈 S z ( r )〉 in the lowest-energy state of ∑ r S z ( r ) = 0 for the Heisenberg model with a local Zeeman field − hS z ( r 0 ) applied to the center site r 0 at the upper edge.…”
Section: Discussionmentioning
confidence: 68%
“…The importance to understand the boundary effects in the Heisenberg model is echoed by plausible edge magnetism in graphene nanoribbons192021222324252627282930. By bottom-up approaches, graphene materials with atomic-sharp zigzag edges have been fabricated successfully.…”
mentioning
confidence: 99%
“…At the same time, however, these results sugggest that the material may be not too far from a possible transition into an ordered state. Other QMC calculations also find sizable charge-density and spin-current correlations, although they do not become long-ranged within the accessible parameter region [31]. Furthermore, a uniform and isotropic strain of about 15% can be expected to induce an interaction-driven metal-insulator transition in graphene [32].…”
Section: Introductionmentioning
confidence: 99%
“…In fact, a recent paper investigated edge spin polarization for large systems, e.g., 10 4 carbon atoms, and it concluded that if the environment time scale τ env is much shorter than τ qd , the system is pushed into the same classical Néel-like state again and again. As a result, the state cannot decay, which is known as the quantum Zeno effect [89]. Furthermore, our results do not require perfect spin polarization at opposite zigzag edges.…”
Section: Conclusion and Discussionmentioning
confidence: 70%