“…In particular, parametric frequency conversions based on χ (2) optical processes such as second‐harmonic generation (SHG), sum‐frequency generation (SFG), and difference frequency generation (DFG) are essential for numerous photonics techniques, including tunable coherent radiation, [ 1 ] frequency metrology, [ 2–4 ] optical signal processing, [ 5,6 ] optical microscopy, [ 7,8 ] quantum information processing, [ 9,10 ] and quantum metrology. [ 11–13 ] The demonstration of efficient χ (2) optical processes on chip has attracted tremendous interest as it holds great promise to enrich the functionality of photonic integrated circuits (PICs) with low power consumption. So far, chip‐scale second‐order nonlinearity has been developed on various material platforms, including lithium niobate (LN) [ 14–24 ] and some III‐V materials [ 25–28 ] with intrinsically possess χ (2) nonlinearity, and silicon [ 29,30 ] and silicon nitride [ 31–33 ] with externally induced χ (2) nonlinearity.…”