We report non-invasive single-charge detection of the full probability distribution Pn of the initialization of a quantum dot with n electrons for rapid decoupling from an electron reservoir. We analyze the data in the context of a model for sequential tunneling pinch-off, which has generic solutions corresponding to two opposing mechanisms. One limit considers sequential "freeze out" of an adiabatically evolving grand canonical distribution, the other one is an athermal limit equivalent to the solution of a generalized decay cascade model. We identify the athermal capturing mechanism in our sample, testifying to the high precision of our combined theoretical and experimental methods. The distinction between the capturing mechanisms allows to derive efficient experimental strategies for improving the initialization.
PACS numbers:The fast formation of quantum dots (QDs) out of a two-dimensional electron system (2DES) constitutes an open problem within the field of nanoscale electronics [1]. The initialization process in these dynamic QDs is a key ingredient in, e.g., devices for quantum information processing [2,3], single-electron current sources [4-6], or nanoelectronic circuits [7,8]. The outcome of the initialization is characterized by a probability distribution P n for trapping exactly n electrons in the QD. The goal is to attain a predictable low dispersion distribution thus making dynamic QDs reliable and reproducible sources of electrons on demand. Deviations from this ideal case may be caused, for instance, by backtunneling [9][10][11] or non-adiabatic excitations [12][13][14].