2018
DOI: 10.26434/chemrxiv.7496627
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Pyramidal Heteroanion-Directed and Reduced MoV-Driven Assembly of Multi-Layered Polyoxometalate Cages

Abstract: The fabrication of redox-active polyoxometalates (POMs) that can switch between multiple states is critical for their application in electronic devices, yet, a sophisticated synthetic methodology is not well developed for such cluster types. Here we describe the heteroanion-directed and reduction-driven assembly of a series of multi-layered POM cages 1-10 templated by 1-3 redox-active pyramidal heteroanions. The heteroanions greatly affect the selfassembly of the resultant POM cages, leading to the generation … Show more

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