“…Among various extraction methodologies developed for uranium capture, the adsorption technique has garnered significant attention due to its cost-effectiveness, straightforward implementation, and impressive efficiency. , To harness the power of this method, the strategic design and fabrication of adsorbents exhibiting stability, rapid kinetics, selectivity, and substantial adsorption capacity serve as fundamental prerequisites . A gamut of adsorption materials, including clays, oxide materials, hydroxyapatite, polymers, graphene oxide, mesoporous silica, carbon materials, and covalent organic frameworks have been explored for uranium separation, − while their applications are often hindered by laborious procedures, sluggish removal rates, and high costs. Metal–organic frameworks (MOFs), as a novel type of porous crystalline materials, have attracted extensive attention due to their expansive surface area, facile tunability, profuse active sites, and ordered pore structure. , These attributes render them exceptional solid-phase adsorbents for radionuclide sequestration, which also facilitates the exploration of structure–function relationships. − So far, numerous strategies have been devised to enhance MOF adsorption performance.…”