Abstract. Point-contact Andreev reflection spectroscopy is used to measure the spin polarization of metals but analysis of the spectra has encountered a number of serious challenges, one of which is the difficulty to distinguish the effects of spin polarization from those of the finite lifetime of Cooper pairs. We have recently confirmed the polarization-lifetime ambiguity for NbCo and Nb-Cu contacts and suggested to use Fermi surface mismatch, the normal reflection due to the difference of Fermi wave vectors of the two electrodes, to solve this dilemma. Here we present further experiments on contacts between superconducting Nb and the ferromagnets Fe and Ni as well as the noble metals Ag and Pt that support our previous results. Our data indicate that the Nb -normal metal interfaces have a transparency of up to about 80% and a small, if not negligible, spin polarization.
IntroductionWith the growing interest in spintronics, measuring the spin polarization P of a metal has become an important task [1]. Andreev reflection spectroscopy of point contacts has been suggested as an effective and versatile technique for measuring the polarization of metals in contact with a superconductor [2,3]. To extract the polarization, one analyses the measured differential resistance spectra with the help of a modified BTK model [4,5,6]. This method has been applied to a wide range of materials, delivering converging values for the spin polarization. The extracted P has a linear or parabolic dependence on the relative strength of the interface barrier Z, and the true value of the polarization P is measured in the Z = 0 limit. Unfortunately, this procedure has also encountered problems, including inadequately understood additional spectral features [7] and, most of all, the degeneracy of the results of the various BTK type models [8,9]. This applies especially when the polarization is low.We have recently demonstrated how difficult it is to distinguish the effects of polarization and finite lifetime of Cooper pairs in the spectra of Nb-Co and Nb-Cu contacts [10]. The finite lifetime of the Cooper pairs has been used to describe the spectra of non-magnetic contacts [11], but with few exceptions [8,9,12] it has not generally been applied to contacts with magnetic metals even though one should expect strong pair breaking in that case. Since spectra of both magnets and non-magnets can often be fitted rather well with the two models, we have suggested