Proton-Coupled-Electron Transfer Enhances the Electrocatalytic Reduction of Nitrite to NO in a Bioinspired Copper Complex
Mark Symes,
Giacomo Cioncoloni,
Isolda Roger
et al.
Abstract:The selective and efficient electrocatalytic reduction of nitrite to nitric oxide (NO) is of tremendous importance, both for the development of NO-release systems for biomedical applications and for the removal of nitrogen oxide pollutants from the environment. In nature, this transformation is mediated by (among others) enzymes known as the copper-containing nitrite reductases. The development of synthetic copper complexes that can reduce nitrite to NO has therefore attracted considerable interest. However, t… Show more
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