Probing the evolution in catalytic graphitization of biomass-based materials for enduring energetic applications

Mennani, Mehdi; Ait Benhamou, Anass; Mekkaoui, Ayoub Abdelkader; El Bachraoui, Fatima; El Achaby, Mounir; Moubarik, Amine; Kassab, Zineb

doi:10.1039/d3ta07449h

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J. Mater. Chem. A

2024

DOI: 10.1039/d3ta07449h

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Probing the evolution in catalytic graphitization of biomass-based materials for enduring energetic applications

Mehdi Mennani,

Anass Ait Benhamou,

Ayoub Abdelkader Mekkaoui

et al.

Abstract: Catalytic processing of biomass and its derivatives to produce graphitizable materials offers a transformative method for converting renewable resources into bio-energy and valuable carbon-based materials.

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Cited by 5 publications

References 88 publications

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Sucrose‐Based Dense, Pure, and Highly‐Crystalline Graphitic Materials for Lithium‐Ion Batteries

Jurkiewicz,

Liszka,

Gancarz

et al. 2024

Adv Funct Materials

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At present, most synthetic graphite materials commonly used as anode active ingredients in lithium‐ion cells are produced by graphitization of petroleum cokes. The carbon footprint associated with synthetic graphite production is significant. Thus, bio‐derived and cheap precursors, such as saccharides, would be an attractive alternative for the sustainable production of graphitic carbons. However, they are non‐graphitizing at temperatures as high as 3000 °C, preserving the curved, fullerene‐like structure of graphene layers and microporosity. Consequently, many lithium ions are consumed during the formation of solid electrolyte interphase films and passivated in the nanovoids. Here, a method for the production of pure, crystalline, graphitic materials based on sucrose disposed of microporosity is presented, which also works with a variety of saccharides and other organic precursors of hard carbons—generally considered incapable of such transformation. This process employs catalytic graphitization by Si particles at high temperatures. The electrochemical response of such derived sucrose‐based graphite in Li‐ion half‐cells demonstrated its feasibility to serve as an anode active material for rechargeable Li‐ion batteries.

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Sucrose‐Based Dense, Pure, and Highly‐Crystalline Graphitic Materials for Lithium‐Ion Batteries

Jurkiewicz,

Liszka,

Gancarz

et al. 2024

Adv Funct Materials

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Boron-doped polyhedral graphite catalyzed by h-BN via structural induction for lithium storage

Wang,

Yang,

Wang

et al. 2024

Carbon

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Biocarbon graphenization processes and energy assessment. A review

Rigollet,

Weiss-Hortala,

Flamant

et al. 2024

Chemical Engineering Journal

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Probing the evolution in catalytic graphitization of biomass-based materials for enduring energetic applications

Abstract: Catalytic processing of biomass and its derivatives to produce graphitizable materials offers a transformative method for converting renewable resources into bio-energy and valuable carbon-based materials.

Cited by 5 publications

References 88 publications

Sucrose‐Based Dense, Pure, and Highly‐Crystalline Graphitic Materials for Lithium‐Ion Batteries

Sucrose‐Based Dense, Pure, and Highly‐Crystalline Graphitic Materials for Lithium‐Ion Batteries

Boron-doped polyhedral graphite catalyzed by h-BN via structural induction for lithium storage

Biocarbon graphenization processes and energy assessment. A review

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