SummaryThe Szilard-Chalmers reaction has been developed as a sensitive detector for the comparison of neutrons from sources of different primary energy and angular distribution. Using sodium permanganate solution, a detection efficiency of approximately 7 per cent. for all neutrons in the energy range 0--5 MeV was obtained and high accuracy achieved.The method of detection was employed to make the following measurements: {i) The neutron yield from the spontaneous fission of natural uranium was found to be (I· 56±0·12) X 10-2neutrons sec-1 g-l.(ii) The cross section for the reaction 6Li(y, n) at 6·2 MeV was found to be (3±2) X 10-28 cm 2 . (iii) The cross section for the reaction "Be(n, 2n) induced by Ra-Be and Po-Be sources of neutrons was found to be (0·37±0·06) X 10-2 • cm 2 . (iv) A limit was placed on the cross-over transition from the 2·5 MeV state to the ground state in 60CO. The transition probability was found to be less than 1 X 10-6 of that for the cascade consisting of the two y-rays.