“…31,32 QOC constitutes a powerful tool for manipulating the dynamics of quantum systems, 28,32,33 including the control of qubits, 34 population of vibrational states, 35 and coupled spin dynamics, 36 among others. Regarding molecular orientation control, the Krotov algorithm 31,37,38 is used to design terahertz laser pulses, 39 or to manipulate the permanent dipole orientation of molecular ensembles, as reported in various studies. [40][41][42][43] In addition, this algorithm has been used to optimize alignment of molecules immersed in a thermal bath.…”