“…[2][3][4] Up to present, a lot of research papers on KNNbased lead-free piezoelectric ceramics have been published, including the piezoelectric properties, [5][6][7] the energy-storage properties, 8 etc. In order to further improve the piezoelectric properties of KNN, engineering of the polymorphic phase transition (PPT) between tetragonal and orthorhombic phases, i.e., shifting downward the PPT point T OÀT to ambient temperature through chemical modifications, 9 has been employed, represented by the formation of pseudobinary solid solutions between KNN and one additional component, e.g., KNN-LiTaO 3 , 10-14 KNN-LiSbO 3 15-17 KNN-BiFeO 3 18 and so on.…”