Chlorine-containing halocarbons, such as chloromethane (CH 3 Cl), chloroform (CHCl 3 ), and chlorofluorocarbons (CFCs), can photo-dissociate in the stratosphere, releasing reactive chlorine radicals that catalyze ozone depletion. Among the naturally produced atmospheric chlorocarbons, CHCl 3 is the second-largest natural carrier of chlorine after CH 3 Cl. With an average tropospheric lifetime of 149 days (Engel et al., 2018), it is categorized as a very short-lived substance (VSLS). Hence, the ozone-depleting capacity of CHCl 3 was thought to be minor and was not regulated by the Montreal Protocol. However, observations over the past decade showed its atmospheric molar fractions have been steadily increasing (Engel et al., 2018;Fang et al., 2019). Numerical model simulations also indicated the recovery of stratospheric ozone may be significantly delayed if atmospheric concentrations of VSLSs, including CHCl 3 , continue to grow (Fang et al., 2019).Natural sources of CHCl 3 are believed to predominate over anthropogenic sources, accounting for 50%-90% of global CHCl 3 emissions (McCulloch, 2003;Worton et al., 2006). The natural emissions of CHCl 3 are