Samples of POCl 3 -SnCl 4 -235 UO 2 -Dy 3+ solutions have been prepared to investigate conversion of energy of heavy charged particles into optical radiation. Experimental data on radioluminescent charac teristics of Dy 3+ upon homogenous excitation of solutions by uranium α radiation have been obtained. The efficiency of conversion of the energy of uranium α particles into light energy depends on the Dy 3+ concen tration and the Dy3+ luminescence lifetime τ. At [Dy 3+ ] = 0.2 mol/L and τ = 550 μs, the conversion effi ciency is 0.12 ± 0.01% for the luminescent transition 4F 9 /2 → 6H 13 /2 (λ max = 574 nm) or 0.20 ± 0.01% for the visible and near IR regions of Dy3+ luminescence.