“…27 Since ME materials show an interesting interplay between the magnetic and electric properties of the matter, 28,29 those materials have drawn increasing interest due to their potential applications in areas such as information storage, spintronics, sensors, and actuators, among others. 24,30,31 ME materials can also reveal an important magnetodielectric (MD) coupling, 32 applied magnetic field, expanding the range of applications to tunable filters or four-state memories, among others. 17,33 In this work, composite films with 0−3 connectivity were prepared via in situ polymerization, using spherical cobalt ferrite nanoparticles (CoFe 2 O 4 ) as fillers and amorphous copolyimides, based on 3-bis(3-aminophenoxy)benzene (diamine 0CN) and 1,3-bis-2-cyano-3-(3-aminophenoxy)phenoxybenzene (diamine 2CN), as polymer matrix (Figure 1).…”