Abstract:We propose and demonstrate a hybrid photonic-plasmonic nanolaser that combines the light harvesting features of a dielectric photonic crystal cavity with the extraordinary confining properties of an optical nano-antenna. For this purpose, we developed a novel fabrication method based on multi-step electron-beam lithography. We show that it enables the robust and reproducible production of hybrid structures, using a fully top-down approach to accurately position the antenna. Coherent coupling of the photonic an… Show more
“…Sophisticated slotted waveguides [141,[151][152][153] as well as nanobeam cavities [140,146,150,[154][155][156][157][158][159][160] have also been implemented for analyte-specific stoichiometric studies and biomolecule micromanipulation. Extreme, sub-attomolar detection of a streptavidin protein was reported for nanoslot PhC nanolasers [139,[161][162][163][164][165][166][167][168], while novel PhC nanocavities combined with plasmonic nanostructures have emerged as hybrid photonic-plasmonic biosensors [169][170][171][172][173][174][175][176][177][178][179]. Unusually sensitive biodetection down to the single-molecule level with nanostructured materials comprising selfassembled silver nanoparticles on PhC diatom biosilica [180,181] and a gold antenna-in-a-nanocavity [182] substantiates the fast and steady advancement of hybrid photonic-plasmonic instrumentation utilising PhCs.…”
Section: Photonic Crystals Engineered With Nano/microcavities For Intmentioning
confidence: 99%
“…Computational analysis pinpointed parameters/dimensions for an ultrahigh Q/V ratio and hence conditions conducive for trapping and micromanipulation. The experimental realisation of a hybrid nanolaser that uses the coupling between a LSPR of a bowtie and photonic mode of an active PhC with a L7 microcavity is visible in Figure 30C-H [179]. The fabrication approach is also flexible in terms of variability of scale and morphology as is demanded by the constraints imposed by the analyte.…”
Section: Photonic Crystals Engineered With Nano/microcavities For Intmentioning
confidence: 99%
“…Here, the (G) normalised lasing spectra and (H) peak versus optical pump power are plotted. Adapted from [179]. Figure 34D and E as well as normal dsDNA and XPA in Figure 34F and G [182].…”
Nanophotonic device building blocks, such as optical nano/microcavities and plasmonic nanostructures, lie at the forefront of sensing and spectrometry of trace biological and chemical substances. A new class of nanophotonic architecture has emerged by combining optically resonant dielectric nano/microcavities with plasmonically resonant metal nanostructures to enable detection at the nanoscale with extraordinary sensitivity. Initial demonstrations include single-molecule detection and even single-ion sensing. The coupled photonic-plasmonic resonator system promises a leap forward in the nanoscale analysis of physical, chemical, and biological entities. These optoplasmonic sensor structures could be the centrepiece of miniaturised analytical laboratories, on a chip, with detection capabilities that are beyond the current state of the art. In this paper, we review this burgeoning field of optoplasmonic biosensors. We first focus on the state of the art in nanoplasmonic sensor structures, high quality factor optical microcavities, and photonic crystals separately before proceeding to an outline of the most recent advances in hybrid sensor systems. We discuss the physics of this modality in brief and each of its underlying parts, then the prospects as well as challenges when integrating dielectric nano/microcavities with metal nanostructures. In Section 5, we hint to possible future applications of optoplasmonic sensing platforms which offer many degrees of freedom towards biomedical diagnostics at the level of single molecules.
“…Sophisticated slotted waveguides [141,[151][152][153] as well as nanobeam cavities [140,146,150,[154][155][156][157][158][159][160] have also been implemented for analyte-specific stoichiometric studies and biomolecule micromanipulation. Extreme, sub-attomolar detection of a streptavidin protein was reported for nanoslot PhC nanolasers [139,[161][162][163][164][165][166][167][168], while novel PhC nanocavities combined with plasmonic nanostructures have emerged as hybrid photonic-plasmonic biosensors [169][170][171][172][173][174][175][176][177][178][179]. Unusually sensitive biodetection down to the single-molecule level with nanostructured materials comprising selfassembled silver nanoparticles on PhC diatom biosilica [180,181] and a gold antenna-in-a-nanocavity [182] substantiates the fast and steady advancement of hybrid photonic-plasmonic instrumentation utilising PhCs.…”
Section: Photonic Crystals Engineered With Nano/microcavities For Intmentioning
confidence: 99%
“…Computational analysis pinpointed parameters/dimensions for an ultrahigh Q/V ratio and hence conditions conducive for trapping and micromanipulation. The experimental realisation of a hybrid nanolaser that uses the coupling between a LSPR of a bowtie and photonic mode of an active PhC with a L7 microcavity is visible in Figure 30C-H [179]. The fabrication approach is also flexible in terms of variability of scale and morphology as is demanded by the constraints imposed by the analyte.…”
Section: Photonic Crystals Engineered With Nano/microcavities For Intmentioning
confidence: 99%
“…Here, the (G) normalised lasing spectra and (H) peak versus optical pump power are plotted. Adapted from [179]. Figure 34D and E as well as normal dsDNA and XPA in Figure 34F and G [182].…”
Nanophotonic device building blocks, such as optical nano/microcavities and plasmonic nanostructures, lie at the forefront of sensing and spectrometry of trace biological and chemical substances. A new class of nanophotonic architecture has emerged by combining optically resonant dielectric nano/microcavities with plasmonically resonant metal nanostructures to enable detection at the nanoscale with extraordinary sensitivity. Initial demonstrations include single-molecule detection and even single-ion sensing. The coupled photonic-plasmonic resonator system promises a leap forward in the nanoscale analysis of physical, chemical, and biological entities. These optoplasmonic sensor structures could be the centrepiece of miniaturised analytical laboratories, on a chip, with detection capabilities that are beyond the current state of the art. In this paper, we review this burgeoning field of optoplasmonic biosensors. We first focus on the state of the art in nanoplasmonic sensor structures, high quality factor optical microcavities, and photonic crystals separately before proceeding to an outline of the most recent advances in hybrid sensor systems. We discuss the physics of this modality in brief and each of its underlying parts, then the prospects as well as challenges when integrating dielectric nano/microcavities with metal nanostructures. In Section 5, we hint to possible future applications of optoplasmonic sensing platforms which offer many degrees of freedom towards biomedical diagnostics at the level of single molecules.
“…One of their interesting features is their ability to focus light at the nanometer scale, leading to strong local fields (called hot spots) near the metal surfaces [4,5]. The fact that the energy of LSPRs can be tuned through variation of the shape, the size, the composition, or the environment of the metal NPs [3,6,7] has opened the way to applications within the domains of biosensing [8], Raman spectroscopies [9,10], solar cells [11], near-field imaging [12], enhanced fluorescence spectroscopy [9], and nanolasers [13]. In addition, plasmonic excitations often play an important part in optical metamaterials [14][15][16][17][18][19][20][21][22][23][24][25][26][27][28][29][30][31][32][33] (i.e., artificially structured materials with a unit structure considerably smaller than the wavelength of visible light [34]), like those in negative optical index materials [14,15], materials for superresolution applications [17][18][19][20], and electromagnetic cloaks [21].…”
We study the evolution of the surface-plasmon resonances of individual ion-beam-shaped prolate gold nanoparticles embedded in a dielectric SiO 2 environment by electron-energy-loss spectroscopy mapping in a scanning transmission electron microscope. The controlled symmetric dielectric environment obtained through the ion-beam-shaping method allows a direct quantitative comparison with numerical results obtained through simulations (auxiliary differential-equation finite-difference time-domain and boundary-element method) and with theoretical results obtained through analytical models (quasistatic model for prolate nanoellipsoids and waveguide model for infinite one-dimensional plasmonic waveguides), with which our experimental results are in very good agreement. We confirm the accuracy of state-of-the-art numerical tools and analytical theories that establish ion-beam shaping as a very promising method to design metal-dielectric nanocomposites with well-predicted optical properties, and with many possible applications in surfaceenhanced Raman spectroscopy and second-harmonic generation, as well as in conventional applications of metamaterials like negative refraction, superimaging, and invisibility cloaking.
“…Hybrid plasmonic-photonic devices were reported in 2014 for lasing (Zhang et al 2014) and light matter coupling (Michael et al 2010). In 2014, ODell et al reported a technique for assembling photonic-plasmonic nanotweezers by optically guiding multiwalled carbon nanotubes to attach them onto a silicon waveguide (ODell et al 2014).…”
We investigate the use of a hybrid nanoresonator comprising a photonic crystal (PhC) cavity coupled to a plasmonic bowtie nanoantenna (BNA) for the optical trapping of nanoparticles in water. Using finite-difference time-domain simulations, we show that this structure can confine light to an extremely small volume of $ 30; 000 nm 3 ð $ 30 zl) in the BNA gap whilst maintaining a high quality factor (5400-7700). The optical intensity inside the BNA gap is enhanced by a factor larger than 40 compared to when the BNA is not present above the PhC cavity. Such a device has potential applications in optical manipulation, creating high precision optical traps with an intensity gradient over a distance much smaller than the diffraction limit, potentially allowing objects to be confined to much smaller volumes and making it ideal for optical trapping of Rayleigh particles (particles much smaller than the wavelength of light).
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