“…Based on Maxwell‐Garnett theory, lot of (e.g. 40 wt%) high‐ k nanofillers, such as Pb(Zr1‐xTix)O 3 , BaTiO 3 , SrTiO 3 , SiO 2 and TiO 2 [12–19], should be added into the polymer matrix to enhance the dielectric constant, resulting in deteriorating the flexibility and processability of the nanocomposites. According to Maxwell–Wagner–Sillars Polarisation Theory, when the volume fraction of electrically conductive nanofiller is close to but lower than the percolation threshold, the dielectric constant of the nanocomposites is obviously improved microcapacitors and space charge polarisation [20, 21], such as Ag, Ni, Fe, Fe 3 O 4 , Zn, ZnO, carbon nanotubes (CNTs) and graphene nanosheets [22–29].…”