“…13,14 PSM works with crystals [13][14][15][16][17][18][19] and with thin films. [20][21][22][23] PSM has also been used to image domains 14,24 thermally written polarization patterns, [25][26][27][28] and to follow polarization and domain dynamics. [29][30][31][32] Moreover, 3D polarization information can be obtained from crystals and thick films by combining 2D laser scanning with depth profiles obtained using either pulse time-of-flight methods, 33 or Laser Intensity Modulation Method (LIMM), [34][35][36][37][38] or both.…”
“…13,14 PSM works with crystals [13][14][15][16][17][18][19] and with thin films. [20][21][22][23] PSM has also been used to image domains 14,24 thermally written polarization patterns, [25][26][27][28] and to follow polarization and domain dynamics. [29][30][31][32] Moreover, 3D polarization information can be obtained from crystals and thick films by combining 2D laser scanning with depth profiles obtained using either pulse time-of-flight methods, 33 or Laser Intensity Modulation Method (LIMM), [34][35][36][37][38] or both.…”
“…The depth-resolution is typically less than 1 µm, and near-surface lateral resolutions of less than 40 µm have been reported [2]. Closely related techniques are the focused or scanning "Laser Intensity Modulation Method" (LIMM) [3,4] and pyroelectric microscopy [5]. Recently, a multi-beam-point analysis that couples the current signal from several neighboring spots resulted in a 2-4 improvement in the lateral resolution [6].…”
Fig. 1: Experimental setup for three-dimensional polarization profiling. The diode laser can be replaced with a 532 nm frequency-doubled Nd:YAG laser.Abstract-Thermal-pulse tomography (TPT) has been shown to be a valuable tool for non-destructively measuring threedimensional electrical polarization and space-charge distributions in electret polymers. However, one of its drawbacks is the high thermal stress imposed on the sample surface when short pulses of laser light are focused to a tight spot. Q-switched Nd:YAG lasers, which are frequently used as heat source in TPT experiments, have a pulse duration of approximately 5 ns. However, due to bandwidth limitations of the amplifier circuits, the stimulating heat pulse can be as long as a few µs without significant loss of depth resolution. Recently, high-power diode lasers have become available that can be electrically driven to provide light pulses of the desired length. The longer light pulses from the diode laser have a significantly lower peak power density, thus avoiding ablation damage to the electrode, even at higher pulse energies. We present spatially resolved polarization maps of poly(vinylidene-trifluoroethylene) samples showing the significantly enhanced signal-to noise ratio of the upgraded instrument.
“…The PSM method has proven useful for studying domains and other polarization inhomoge neities in ferroelectric crystals [11,15], ferroelectric poly mer thin films [9,16,17], and periodically poled non linear optical polymer films [18,19]. The PSM method consists of heating a small area of the capacitor with a laser beam, in this case the 5 mW output of a 633 nm he lium-neon laser that was focused to a 17-μm diameter spot with a microscope objective.…”
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