Physico-chemical principles of AC electrosynthesis
Yong Rui Poh,
Joel Yuen-Zhou
Abstract:Electrolysis integrates renewable energy into chemical manufacturing and is key towards sustainable chemistry. Controlling the waveform beyond direct current addresses the long-standing obstacle of chemoselectivity, yet it also expands the parameter set to optimise, creating a demand for theoretical predictions. Here, we report the first analytical theory for predicting chemoselectivity in alternating current electrosynthesis. The mechanism is a selective reversal of the unwanted redox reaction during periods … Show more
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