2020
DOI: 10.1039/c9cs00560a
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Photoexcited carrier dynamics in colloidal quantum dot solar cells: insights into individual quantum dots, quantum dot solid films and devices

Abstract: Topics of photoexcited carrier dynamics in quantum dot solar cells are reviewed and discussed for the first time.

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Cited by 85 publications
(64 citation statements)
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“…The Nyquist plot fitting results of BTPA-7 based PSC device exhttps://engine.scichina.com/doi/10.1016/j.jechem.2020.02.021 hibit both a larger R s (30 ) and a lower R rec (220 ), which may arise from the lower conductivity of the BTPA-7 layer. These results corroborate the lower FF and V oc values of BTPA-7 based PSC as shown in the J-V curves compared with the spiro-OMeTAD reference PSC device [46] . Stability is the challenge for the PSC commercialization [47 , 48] .…”
Section: Resultssupporting
confidence: 85%
“…The Nyquist plot fitting results of BTPA-7 based PSC device exhttps://engine.scichina.com/doi/10.1016/j.jechem.2020.02.021 hibit both a larger R s (30 ) and a lower R rec (220 ), which may arise from the lower conductivity of the BTPA-7 layer. These results corroborate the lower FF and V oc values of BTPA-7 based PSC as shown in the J-V curves compared with the spiro-OMeTAD reference PSC device [46] . Stability is the challenge for the PSC commercialization [47 , 48] .…”
Section: Resultssupporting
confidence: 85%
“…Similarly, Yang et al [ 38 ] studied a similar photodevice as a photodetector reporting V oc = 1.2–1.3 V and J sc of 1–4 mA cm −2 . It should be noted that the MPA ligand may result in a different electronic work function, as demonstrated for PbS QD solids, in which the work function can vary several hundreds of meVs depending on the ligand post-treatment applied [ 17 , 39 ].…”
Section: Resultsmentioning
confidence: 99%
“…Therefore, more efforts are still needed to design and prepare different types of MHP photocatalysts to fully explore their potentials in photocatalysis. The proposed directions for future research on MHP-based photocatalysts are: (i) Utilization of MHPs with different morphologies [91], such as QDs, nanorod, and 2D nanosheet to facilitate the charge separation and mass transport; (ii) rational design of MHP-based composites to achieve stronger light absorption and promote charge separation; (iii) precise control of charge carriers in MHPs with the aid of modern characterization methods, such as transient absorption and time-resolved terahertz spectroscopy [195]; (iv) preparation of stable and eco-friendly highperformance MHP-based photocatalysts; (v) investigation of mechanisms by combining theoretical calculations and in-situ characterization techniques to probe the reaction pathways and reveal the changes of catalysts during photocatalysis [196]. These challenges also signify great opportunities for further improving photocatalytic activity and exploring more potential reactions in MHPs.…”
Section: Discussionmentioning
confidence: 99%