Abstract:The photodissociation spectroscopy of weakly bonded bimolecular complexes can give important insight into fundamental molecular interactions and dynamics. We have applied these techniques to a study of metal ion-ethylene interactions in the Mg\3s)-C2H4and At(3s 2)-C 2H4 rt-bonded complexes. Experimental work is supported by ab-initio electronic structure calculations. These experiments allow us to explore and compare the chemical binding, electronic structure, and nonadiabatic dissociation dynamics of these co… Show more
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