Photocatalytic Synthesis of Ammonia from Hollow Coral-Like Graphitic Carbon Nitride/FeOCl Loaded with Fe-1T MoS2 Nanosheets as Cocatalysts
Fushan Wen,
Shichuang Liu,
Xiaoli Huang
et al.
Abstract:Photocatalytic
ammonia synthesis (PAS) represents an emerging environmentally
friendly approach to ammonia production. In this work, we employed
Fe doping to modify the cocatalyst 1T MoS2, enhancing the
active N2 sites on Fe-1T MoS2 by inducing defects
on the surface of 1T MoS2. Afterward, Fe-1T MoS2 was loaded onto a hollow coral-like graphitic carbon nitride (CCN)/FeOCl
composite. Under simulated sunlight, the efficiency of 5% Fe-1T MoS2@CCN/FeOCl (Fe-MCN/FeOCl) reached 367.62 μmol g–1 h–1, surpassing 1T MoS… Show more
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