Photo‐induced Cobalt‐catalyzed Aerobic N−N Coupling of Diarylamines at Room Temperature

Luo, Guangzhong; Han, Yu; Zhang, Ruohan; Ding, Dongmiao; Dian, Longyang

doi:10.1002/ajoc.202200553

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Catalytic N–n Bond Formation1

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2023

2024

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“…Through the combination of photocatalysis and transition-metal catalysis, Dian and co-workers realized a cobalt-catalyzed N–N coupling of diarylamines (Scheme ). With Co(OAc) 2 ·4H 2 O as the catalyst and diphenyl-1,10-phenanthroline ( Bphen ) as the ligand, tetraphenylhydrazines 17 could be formed in moderate to good yields when the reaction was irradiated at 390–395 nm.…”

Section: Catalytic N–n Bond Formationmentioning

confidence: 99%

Recent Advances in Catalytic Nitrogen–Nitrogen Bond Formation Reactions

Hu,

Wu,

Gao

et al. 2024

ACS Catal.

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The lack of effective strategies for direct construction of nitrogen−nitrogen bonds has hampered developments in the synthesis and application of molecules containing hydrazine or azo motifs. Attracted by their properties both in material science and in medicinal chemistry, more and more attention has been drawn to this area, resulting in fast growth in the design and synthesis of azaheterocycles and substituted hydrazines. This review focuses on efficient catalytic approaches toward the formation of N−N and N�N bonds through different strategies, including oxidative dehydrogenation, nitrene-transfer reaction, reductive coupling, and some other recently developed methods.

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Section: Catalytic N–n Bond Formationmentioning

confidence: 99%