2011
DOI: 10.1143/jpsj.80.064704
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Phonon Dispersion and Electron–Phonon Interaction in Peanut-Shaped Fullerene Polymers

Abstract: We reveal that the periodic radius modulation peculiar to one-dimensional (1D) peanut-shaped fullerene (C60) polymers exerts a strong influence on their low-frequency phonon states and their interactions with mobile electrons. The continuum approximation is employed to show the zonefolding of phonon dispersion curves, which leads to fast relaxation of a radial breathing mode in the 1D C60 polymers. We also formulate the electron-phonon interaction along the deformation potential theory, demonstrating that only… Show more

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Cited by 13 publications
(14 citation statements)
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References 40 publications
(67 reference statements)
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“…It has been known that mobile electrons whose motion is confined to a two-dimensional, curved thin layer behave differently from those on a conventional flat plane because of an effective electromagnetic field [ 159 , 160 , 161 , 162 , 163 , 164 ] that can affect low-energy excitations of the electrons. Associated variations in the electron-phonon coupling [ 165 ] and phononic transport [ 166 ] through the deformed nano-carbon materials are also interesting and relevant to the physics of radially corrugated MWNTs.…”
Section: Radial Compression Bucklingmentioning
confidence: 99%
“…It has been known that mobile electrons whose motion is confined to a two-dimensional, curved thin layer behave differently from those on a conventional flat plane because of an effective electromagnetic field [ 159 , 160 , 161 , 162 , 163 , 164 ] that can affect low-energy excitations of the electrons. Associated variations in the electron-phonon coupling [ 165 ] and phononic transport [ 166 ] through the deformed nano-carbon materials are also interesting and relevant to the physics of radially corrugated MWNTs.…”
Section: Radial Compression Bucklingmentioning
confidence: 99%
“…The remarkable consistency between theory and experiment tells us that the confining potential approach is effective to explore the geometryproperty relations in C60 polymers and possibly other curved nanomaterials. In addition to the shift in the TLL exponent, C60 polymers are expected to have distinct features far from conventional nano-carbons, in view of the electron-phonon interaction 17) and the resulting charge-density-wave states, 18) even though they remain to be verified in experiments.…”
Section: Tll Exponent Shift In C60 Polymersmentioning
confidence: 99%
“…An overall agreement between the theory and the experiments is obtained by assuming p ∼ 0.3. The other parameters we used are TA = 220 cm −1 , h = 360 cm −1 , and 2 (0) = 360 K; the first two values were estimated from the phonon model for 1D C 60 polymers, 31 and the last value gives 2 (0)/k B T c = 6 consistent with many CDW compounds. 32 The generality of Eq.…”
Section: B Comparison With Experimental Datamentioning
confidence: 99%