Received Month X, XXXX; revised Month X, XXXX; accepted Month X, XXXX;posted Month X, XXXX (Doc. ID XXXXX); published Month X, XXXXWe present a highly efficient source for discrete frequency-entangled photon pairs based on spontaneous parametric downconversion using 3 rd order type-0 quasi-phase matching in a periodically poled MgO-doped stoichiometric LiTaO3 crystal pumped by a 355.66 nm laser. Correlated two-photon states were generated with automatic conservation of energy and momentum in two given spatial modes. These states have a wide spectral range, even under small variations in crystal temperature, which consequently results in higher discreteness. Frequency entanglement was confirmed by measuring twophoton quantum interference fringes without any spectral filtering.Entangled photon pairs are a very important resource in the field of quantum information science. Over the last three decades, various types of entangled photon-pair sources have been developed not only to study the foundation of quantum mechanics but also to implement real world quantum technologies [1,2]. Among them, polarization-entangled pairs of photons have been adopted as the most versatile light source because their polarization has a well-defined orthogonal basis, and which can be easily manipulated using only linear optics [3,4]. In combination with the polarization degree of freedom, the frequency (or wavelength) of a single photon can also be employed as a basic unit to prepare a quantum state [5][6][7][8][9][10]. Particularly, generation and manipulation of the multi-dimensional quantum states by utilizing frequency degree of freedom is one of the interesting issues for potential applications in practical quantum communication system [11][12][13][14]. To utilize the frequency degree of freedom as a quantum information resource, it is necessary to separate the center frequencies of the two photons over a range substantially larger than the spectral bandwidth of the two individual photons.Recently, certain types of photonic sources for discrete frequency-entangled states using correlated photon pairs were reported and used to explore the potential applications in quantum information and communication technologies. In the first experimental demonstration, Ramelow and co-workers reported a discrete tunable frequency-entangled photon-pair source generated by spontaneous parametric down-conversion (SPDC) using type-II collinear quasi-phase matching (QPM) in a periodically poled KTiOPO4 (PPKTP) crystal inside a polarization Sagnac interferometer [5,6]. To successfully obtain frequency symmetric states in the two spatial modes, they used a method of transferring the polarization entanglement onto a frequency-entangled state. Further work was performed using optical fibers, such as a dispersion shifted fiber [7,8] and a commercial polarization-maintaining fiber [9], to generate frequencyentangled photon-pair states via spontaneous four-wave mixing (SFWM). Occasionally, fiber sources have inevitably required cumbersome cooling systems to ...