“…Additionally, TE couples with different TE materials may have different optimum S p / S n values, and four typical materials (Figure S2) are selected for simulation, including BiTe‐based 29 alloys ( T h = 500 K, T c = 300 K), p‐type 30 and n‐type 31 PbTe‐based alloys ( T h = 700 K, T c = 350 K), p‐type 32 and n‐type 33 SiGe‐based alloys ( T h = 1000 K, T c = 500 K), p‐type NbFeSb‐based half‐Heusler alloys, 34 and n‐type CoSb‐based half‐Heusler alloys 35 ( T h = 1000 K, T c = 500 K). Here, the representative data of the Seebeck coefficient, electrical resistivity, and thermal conductivity are selected from the above literature, and these data are obtained by a polynomial fitting method 40,41 . Among these references, some studies only refer to one kind of material; other studies refer to various materials due to the difference in doping concentration and elements, and the better one was adopted in this research.…”