The impact of aerosols on human health
and climate is well-recognized,
yet many studies have only focused on total PM2.5 or changes
from anthropogenic activities. This study quantifies the health and
climate effects of organic aerosols (OA) from anthropogenic, biomass
burning, and biogenic sources. Using two atmospheric chemistry models,
CAM-chem and GEOS-Chem, our findings reveal that anthropogenic primary
OA (POA) has the highest efficiency for health effects but the lowest
for direct radiative effects due to spatial and temporal variations
associated with population and surface albedo. The treatment of POA
as nonvolatile or semivolatile also influences these efficiencies
through different chemical processes. Biogenic OA shows moderate efficiency
for health effects and the highest for direct radiative effects but
has the lowest efficiency for indirect effects due to the reduced
high cloud, caused by stabilized temperature profiles from aerosol–radiation
interactions in biogenic OA-rich regions. Biomass burning OA is important
for cloud radiative effect changes in remote atmospheres due to its
ability to be transported further than other OAs. This study highlights
the importance of not only OA characteristics such as toxicity and
refractive index but also atmospheric processes such as transport
and chemistry in determining health and climate impact efficiencies.