Oxidative Fluorination of a Ternary Cu/ZnO/FeOx Methanol Catalyst─A Proof of Principle
Lukas D. Ernst,
Christian Njel,
Wijnand Marquart
et al.
Abstract:Oxidative fluorination is reported to increase methanol (MeOH) productivity of binary copper−zinc oxide (CZ) catalyst systems yet is incompatible with all the hitherto tested ternary support materials. Here, we show that the oxidative fluorination with F 2 gas of CZ MeOH catalysts including iron oxide as a support material improves catalytic performances. A systematic variation of the compositions of the investigated ternary CZFe (copper, zinc, and iron) catalyst system led to a total of 13 different systems. … Show more
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