It has been shown that the Earth's inner core has an axisymmetric anisotropic structure with seismic waves traveling ∼3% faster along polar paths than along equatorial directions. Hemispherical anisotropic patterns of the solid Earth's core are rather complex, and the commonly used hexagonal-close-packed iron phase might be insufficient to account for seismological observations. We show that the data we collected are in good agreement with the presence of two anisotropically specular east and west core hemispheres. The detected travel-time anomalies can only be disclosed by a lattice-preferred orientation of a body-centered-cubic iron aggregate, having a fraction of their [111] crystal axes parallel to the Earth's rotation axis. This is compelling evidence for the presence of a body-centered-cubic Fe phase at the top of the Earth's inner core.elastic anisotropy | Fe-bcc/-hcp | PKiKP/PKIKP waves | molecular dynamics T he Earth's inner core (IC) is a small spherical body (with a radius of 1,200 km) located at the center of our home planet. Since its discovery in the late 1936 by Inge Lehmann (1), it has long been the most out of reach and enigmatic place of the Earth. Through comparison of the equation of state to seismic data and the abundance of iron, it has been established that the solid IC mainly consists of iron (2-4). The growth of the IC from the freezing of the molten iron alloy at the inner-core boundary (ICB) (5) drives the convection in the outer core and provides the energy source for the geodynamo (6). From the analysis of the normal modes of the Earth's free oscillations and the body wave data, it has been found that compressional P waves travel about 3% faster along the Earth's spin axis than in the equatorial plane (7-10). The growing evidence of an elastic anisotropic IC has continued to generate interesting understandings of the deepest part of our planet, though not all the scientific efforts have converged to the same scenario. Surprisingly, the picture has become more and more confusing as further observations have been collected (7). Explaining the anisotropic IC behavior within a unified and well-accepted geophysical model has become an increasingly complicated issue. Nowadays, we know that the Earth's inner core has a rather complex three-dimensional structure, where texture (11-13) and degree of seismic anisotropy (14-20) change considerably with depth. The most recent view of the solid core corresponds to an uppermost isotropic layer characterized by faster P waves in the eastern hemisphere than in the western one (15,21,22). Although the existence of an outermost isotropic layer has somewhat been questioned (23, 24), more consensus has been reached about the presence of a deeper and more anisotropic region (13,16,25).Different mechanisms have been proposed to explain the IC anisotropy (26, 27), though most of them have firmly relied on the lattice-preferred orientation (LPO) of both the hexagonalclose-packed (hcp) (12,(28)(29)(30)(31) and the body-centered-cubic (bcc) iron crystals (32...