The nonlinear optical limiting and relative nonlinear refractive index in far-field of acid blue29 dye are investigated using radiation of 35mW CW He-Ne laser. It is found that both nonlinear refraction and nonlinear absorption change with decreasing of solvents polarity and varying the input powers.
1-IntroductionWith the extensive use of high-power laser in many different applications, much interest is currently being directed towards the search for new nonlinear optical materials for passive optical limiters used to protect human eyes and solid-state optical sensors from intense laser beams [1][2][3]. Over the past decades, extensive studies on optical limiting materials have been focused on nonlinear organic molecules [4][5], organic dyes [6] and conjugated compounds [7] with respect to nanosecond optical limiting behavior. Nonlinear optical properties of organic dye molecules such as a large nonlinearity, broadband spectral response and fast response time are important for realizing the potential for using organic dyes and their applications in optical limiting and processing fields [8]. Several groups were investigated the concentrations effect on the optical limiting behavior of organic dye molecules [9][10][11][12][13][14][15]. But, several studies were focused on the solvent effect on the optical limiting behavior of organic dye molecules [16][17][18]. The nonlinear absorption mechanism in the dyes is due to reverse saturable absorption (RSA), depending on the change in the absorption in relation with intensity increasing. It is well known that RSA mechanism leads to absorption increase in the sample with increase in intensity which is also explaining the nonlinear optical limiting action in the organic materials [19][20][21]. Following our recent investigations on optical limiting behavior of acid blue29, under excitation of a low power (CW) He-Ne laser irradiation in ethanol only at four different concentrations [9], this paper shows that both nonlinear refraction and nonlinear absorption change with decreasing of solvents polarity and varying the input powers using a 35 mW HeNe laser radiation at 632.8 nm.