One-step synthesis of structural-controlled metal-graphene nanocomposites via flash atomization and plasma-assisted reactions of electrical explosion

Li, Chen; Han, Ruoyu; Bai, Jie; Cao, Yuchen; Yuan, Wei; Wu, Jiawei; Li, Pengfei; Chen, Xi

doi:10.1016/j.carbon.2023.118296

Carbon

2023

DOI: 10.1016/j.carbon.2023.118296

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One-step synthesis of structural-controlled metal-graphene nanocomposites via flash atomization and plasma-assisted reactions of electrical explosion

Chen Li

Ruoyu Han

Jie Bai

et al.

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2024

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Cited by 7 publications

References 45 publications

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Ultra‐Fast Pulsed Discharge Preparation of Coordinatively Unsaturated Asymmetric Copper Single‐Atom Catalysts for CO₂ Reduction

Liu,

Sun,

Chen

et al. 2024

Adv Funct Materials

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Single‐atom catalysts possess great potential for applications in electrochemical carbon dioxide reduction reactions. Recently, the fast and low‐cost preparation of highly efficient single‐atom catalysts remains a challenge. Herein, a high‐density current generated by pulsed discharge is employed for the formation of graphene aerogel anchored Cu single atom catalysts perfectly. The Cu atoms decomposed by Cu(NO3)2•xH2O are fixed on graphene under the local transient high temperature and intense electromagnetic field. The activity and selectivity of formic acid are correlated with the coordinatively unsaturated Cu─N1O1 moieties, reaching an optimal Faradaic efficiency (93.7%) at −0.9 V versus a reversible hydrogen electrode (RHE). In situ characterizations reveal that the asymmetric Cu─N/O structure in a pinched state displays better catalytic activity in CO2RR. Density functional theory results indicate that the Cu─N1O1 sites regulate the adsorption configuration of intermediates and lower the energy barrier for the hydrogenation of *OCHO species, thereby promoting CO2‐to‐HCOOH conversion.

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Ultra‐Fast Pulsed Discharge Preparation of Coordinatively Unsaturated Asymmetric Copper Single‐Atom Catalysts for CO₂ Reduction

Liu,

Sun,

Chen

et al. 2024

Adv Funct Materials

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show abstract

Formation mechanisms of multiple Si/graphene nanocomposites through underwater pulsed discharge using different wire arrangements

Zhong,

Gao,

Qiao

et al. 2024

Ceramics International

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Top-down strategies for achieving high-quality graphene: Recent advancements

Agrawal

2024

Journal of Industrial and Engineering Chemistry

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One-step synthesis of structural-controlled metal-graphene nanocomposites via flash atomization and plasma-assisted reactions of electrical explosion

Cited by 7 publications

References 45 publications

Ultra‐Fast Pulsed Discharge Preparation of Coordinatively Unsaturated Asymmetric Copper Single‐Atom Catalysts for CO₂ Reduction

Ultra‐Fast Pulsed Discharge Preparation of Coordinatively Unsaturated Asymmetric Copper Single‐Atom Catalysts for CO₂ Reduction

Formation mechanisms of multiple Si/graphene nanocomposites through underwater pulsed discharge using different wire arrangements

Top-down strategies for achieving high-quality graphene: Recent advancements

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One-step synthesis of structural-controlled metal-graphene nanocomposites via flash atomization and plasma-assisted reactions of electrical explosion

Cited by 7 publications

References 45 publications

Ultra‐Fast Pulsed Discharge Preparation of Coordinatively Unsaturated Asymmetric Copper Single‐Atom Catalysts for CO2 Reduction

Ultra‐Fast Pulsed Discharge Preparation of Coordinatively Unsaturated Asymmetric Copper Single‐Atom Catalysts for CO2 Reduction

Formation mechanisms of multiple Si/graphene nanocomposites through underwater pulsed discharge using different wire arrangements

Top-down strategies for achieving high-quality graphene: Recent advancements

Contact Info

Product

Resources

About

Ultra‐Fast Pulsed Discharge Preparation of Coordinatively Unsaturated Asymmetric Copper Single‐Atom Catalysts for CO₂ Reduction

Ultra‐Fast Pulsed Discharge Preparation of Coordinatively Unsaturated Asymmetric Copper Single‐Atom Catalysts for CO₂ Reduction