On the theory of charge transport and entropic effects in solvated molecular junctions
Jakub K. Sowa,
Rudolph A. Marcus
Abstract:Experimental studies on single-molecule junctions are typically in need of a simple theoretical approach that can reproduce or be fitted to experimentally measured transport data. In this context, the single-level variant of the Landauer approach is most commonly used but methods based on Marcus theory are also gaining in popularity. Recently, a generalized theory unifying these two approaches has also been developed. In the present work, we extend this theory so that it includes entropic effects (which can be… Show more
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