The connectivity of undersea sensors and airborne nodes across the water-air interface has been long sought. This study designs a free-space wireless laser communications system that yields a high net data rate of 850 Mbit/s when perfectly aligned. This system can also be used for an extended coverage of 1963 cm 2 at the receiver while sustaining a net data rate of 9 Mbit/s over 10 m. The utility of this system was verified for direct communications across the water-air interface in a canal of the Red Sea based on a pre-aligned link as well as a diving pool under a mobile signal-searching mode. The canal deployment measured a real-time data rate of 87 Mbit/s when pre-aligned in turbid water over 50 min, which confirms the system robustness in harsh water environments. In the pool deployment, a drone configured with a photodetector flew over the surface of the water and recorded the underwater signals without a structureassisted alignment. Using a four-quadrature amplitude-modulated orthogonal frequency-division multiplexing (4-QAM-OFDM) modulation scheme provided a net data rate of 44 Mbit/s over a 2.3-m underwater and 3.5-m air link. The results validated the link stability and mitigated problems that arise from misalignment and mobility in harsh environments, which paves the way for future field applications. INDEX TERMS Underwater communication, optical modulation, wireless communications, water-to-air communications, cross-medium communications, mobility I. INTRODUCTION The concept of the Internet of Underwater Things (IoUT) was proposed in 2012 to satisfy the demands of underwater communication networks [1]. The wide, license-free bandwidth and low energy consumption in such environments promote the consideration of underwater wireless optical communication (UWOC) as a transformative technology compared with conventional marine acoustic and radio-frequency (RF) technologies for high-speed communication activities in the IoUT. Verifications of the UWOC physical layer are progressing rapidly [2], with multiple Gbit/s-level UWOC links reported in laboratory studies [3]-[8]. Beyond investigations under ideal laboratory environments, researchers have considered the effects of various natural underwater processes on the performance of UWOC links. Bubbles [9], waves [10], aquatic life [11], water turbidity [12], and oceanic turbulence [13] all degrade communication performance in UWOC by altering the path of light propagation and by inducing misalignment.