Abstract. Volcanic eruptions impact climate through the injection of sulfur dioxide (SO 2 ), which is oxidized to form sulfuric acid aerosol particles that can enhance the stratospheric aerosol optical depth (SAOD). Besides large-magnitude eruptions, Co-injection of 27 Gg HCl causes a lengthening of the SO 2 lifetime and a slight delay in the formation of aerosols, and acts to enhance the destruction of stratospheric ozone and mono-nitrogen oxides (NO x ) compared to the simulation with volcanic SO 2 only. We therefore highlight the need to account for volcanic halogen chemistry when simulating the impact of eruptions such 15 as Sarychev on stratospheric chemistry. The model-simulated evolution of effective radius (r eff ), reflects new particle formation followed by particle growth that enhances r eff to reach up to 0.2 µm on zonal average. Comparisons of the model-simulated particle number and size-distributions to balloon-borne in-situ stratospheric observations over Kiruna, Sweden, in August and September 2009, and over Laramie, U.S.A., in June and November 2009 show good agreement and quantitatively confirms the post-eruption particle enhancement. We show that the model-simulated SAOD is consistent with that derived from OSIRIS 20