Abstract. We investigated the interactions between the air pollutants and
the structure of the urban boundary layer (UBL) over Beijing by using the data
mainly obtained from the 325 m meteorological tower and a Doppler wind lidar
during 1–4 December 2016. Results showed that the pollution episodes in
this period could be characterized by low surface pressure, high relative
humidity, weak wind, and temperature inversion. Compared with a clean daytime
episode that took place on 1 December, results also showed that the
attenuation ratio of downward shortwave radiation was about 5 %, 24 %
and 63 % in afternoon hours (from 12:00 to 14:00 local standard
time, LST) on 2–4 December, respectively, while for the net radiation
(Rn) attenuation ratio at the 140 m level of the 325 m tower was
3 %, 27 % and 68 %. The large reduction in Rn on
4 December was not only the result of the aerosols, but also clouds. Based on
analysis of the surface energy balance at the 140 m level, we found that the
sensible heat flux was remarkably diminished during daytime on polluted
days and even negative after sunrise (about 07:20 LST) till 14:00 LST on 4
December. We also found that heat storage in the urban surface layer played
an important role in the exchange of the sensible heat flux. Owing to the
advantages of the wind lidar having superior spatial and temporal resolution,
the vertical velocity variance could capture the evolution of the UBL well.
It clearly showed that vertical mixing was negatively related to the
concentrating of pollutants, and that vertical mixing would also be weakened
by a certain quantity of pollutants, and then in turn worsened the pollution
further. Compared to the clean daytime on 1 December, the maximums of the
boundary layer height (BLH) decreased about 44 % and 56 % on
2–3 December, when the average PM2.5 (PM1) concentrations in
afternoon hours (from 12:00 to 14:00 LST) were
44 (48) µg m−3 and 150 (120) µg m−3. Part
of these reductions of the BLH was also contributed by the effect of the heat
storage in the urban canopy.