2013
DOI: 10.1103/physrevlett.111.026402
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Observation of ExcitonicN-Body Bound States: Polyexcitons in Diamond

Abstract: We have found a series of resonances associated with the bound state (polyexcitons, PE(N)s) of N excitons up to N=6 in the emission spectra of diamond under two-photon excitation at around 10 K. Time-resolved spectra show a stepwise formation of PE(N)s with smaller to larger N, as well as a successive decay from larger to smaller N. At higher excitation levels, the transformation of PE(N)s into a condensed phase of electron-hole droplets occurs. The binding energies of the PE(N)s, normalized to the exciton Ryd… Show more

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Cited by 31 publications
(28 citation statements)
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“…Recently, a possible signature of Efimov physics in an excitonic system has been claimed to be observed [148]. In reference [148], N -body bound states of excitons, called poly-excitons, have been observed up to N = 6 by a photoluminescence measurement in a diamond crystal. The binding energies of these poly-exciton states were measured, and compared with those found in other crystals [153,154].…”
Section: Universal Few-body Physics With Excitonsmentioning
confidence: 99%
“…Recently, a possible signature of Efimov physics in an excitonic system has been claimed to be observed [148]. In reference [148], N -body bound states of excitons, called poly-excitons, have been observed up to N = 6 by a photoluminescence measurement in a diamond crystal. The binding energies of these poly-exciton states were measured, and compared with those found in other crystals [153,154].…”
Section: Universal Few-body Physics With Excitonsmentioning
confidence: 99%
“…It is also expected to occur in solid-state physics [23,24]. This universality stems from the effective three-body attraction that occurs between particles interacting with nearly resonant short-range interactions.…”
mentioning
confidence: 97%
“…c) (). Although the electron–hole liquid is generally more stable at high density and low temperature, polyexcitons appear under specific density and temperature conditions with a 400–500 ps rise time (). Photo‐injection near the transverse‐acoustic phonon‐assisted absorption edge (hν<5.55eV) of excitons was most effective in reducing the formation of electron–hole droplets and Tex.…”
Section: Electron–hole System In Diamond Under Photo‐injectionmentioning
confidence: 99%
“…Therefore, it is important to understand the exciton diffusivity, free‐carrier mobility, and their relationship. Besides excitons, various complexes such as polyexcitons (), electron–hole plasmas, and electron–hole liquid () are formed in photoexcited diamond, and coexist with excitons in an early time window (<10 ns). We take an advantage of time‐resolved spectroscopy to achieve a temporal and spectral separation of exciton contributions.…”
Section: Introductionmentioning
confidence: 99%