Observation of Dark States in Two-Dimensional Electronic Spectra of Chlorosomes
Vesna Erić,
Xinmeng Li,
Lolita Dsouza
et al.
Abstract:Observations of low-lying dark states in several photosynthetic complexes challenge our understanding of the mechanisms behind their efficient energy transfer processes. Computational models are necessary for providing novel insights into the nature and function of dark states, especially since these are not directly accessible in spectroscopy experiments. Here, we will focus on signatures of dark-type states in chlorosomes, a light-harvesting complex from green sulfur bacteria wellknown for uniting a broad ab… Show more
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