We report on the observation of high-efficiency frequency doubling of 1550 nm continuous-wave laser light in a nonlinear cavity containing a periodically poled potassium titanyl phosphate crystal (PPKTP). The fundamental field had a power of 1:10 W and was converted into 1:05 W at 775 nm, yielding a total external conversion efficiency of 95 AE 1%. The latter value is based on the measured depletion of the fundamental field being consistent with the absolute values derived from numerical simulations. According to our model, the conversion efficiency achieved was limited by the nonperfect mode matching into the nonlinear cavity and by the nonperfect impedance matching for the maximum input power available. Our result shows that cavity-assisted frequency conversion based on PPKTP is well suited for low-decoherence frequency conversion of quantum states of light. © 2011 Optical Society of America OCIS codes: 060.5565, 190.2620. In quantum information science, low-decoherence interfaces are required in order to map quantum information from one system to another. Light at near-infrared frequencies, i.e., around 1550 nm, is well suited to distribute information over standard telecommunication fiber networks with low optical loss [1,2]. For quantum storage devices atomic transitions at around 800 nm are actively researched, in the pulsed as well as in the continuouswave regime [3][4][5]. In order to link these frequency regimes, light at telecommunication wavelengths might be upconverted, e.g., by second harmonic generation (SHG) [6][7][8]. In past years a lot of progress in highefficiency frequency upconversion has been achieved. In [9], a pump depletion of 99% was reported for 50 ns pulses. In [10], a single-photon conversion efficiency of 96% was observed. Here, however, the efficiency of the quantum state transfer was lower than this value due to a 25% background (dark) count rate. For secondharmonic generation of continuous-wave (cw) light [11,12], the highest external conversion efficiency reported so far is 90% [13]. This value also reflects the efficiency of the quantum state transfer since loss due to imperfect matching between input mode and cavity mode of the frequency converter was included and background and dark noise of the detection scheme was negligible.In this Letter, we experimentally investigate the efficiency of cavity-assisted SHG of cw light at 1550 nm in PPKTP. This material is a promising candidate for reaching high quantum state transfer efficiencies, since the optical absorption of the material is low enough to observe up to 12:7 dB of quantum noise squeezing [14]. We are particularly interested in maximizing the external conversion efficiency, as given by the power ratio of the 775 nm cavity output beam and the 1550 nm input beam, i.e., our conversion efficiency value is not artificially increased by inferring to a situation with perfect mode matching into the cavity. In the case of intracavity frequency doubling inside a laser resonator, a value of nearly 100% was recently observed [15]...