Numerical Voltammetry of Phase Separating Materials Using Phase Field Modeling
Umair Hussain,
Narasimhan Swaminathan,
Gandham Phanikumar
Abstract:Higher capacity materials, such as Si and Sn are known to have phase separating behavior during the (de)lithiation. While initial models for lithiation in graphite electrode were based on single phase diffusion, with the introduction of Si and Sn, disposition of the models has shifted to the two-phase diffusion. It is important to understand the interaction of various phenomenon in materials which show phase change during (dis)charging cycles. In this work, we present a phase field model to simulate two-phase … Show more
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