2014
DOI: 10.1103/physrevb.90.075103
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Nonlinear spectroscopy of exciton-polaritons in a GaAs-based microcavity

Abstract: We present a systematic investigation of two-photon excitation processes in a GaAs-based microcavity in the strong-coupling regime. We observe second harmonic generation resonant to the upper and lower polariton level, which exhibits a strong dependence on the photonic fraction of the corresponding polariton. In addition, we have performed two-photon excitation spectroscopy to identify 2p exciton states which are crucial for the operation as a terahertz lasing device, which was suggested recently [A. V. Kavoki… Show more

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Cited by 21 publications
(22 citation statements)
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“…The mechanism of the optical field formation discussed here is related to renormalization of the electron energy spectrum of bulk GaAs in the field of elliptically polarized light wave and to enhancement of the electromagnetic field intensity in microcavities. Besides, semiconductor microcavities demonstrate a variety of specific polarization-dependent linear and nonlinear effects 45 46 47 48 , including polarization conversion, self-induced Larmor precession, second harmonic generation, spin to angular momentum conversion, etc. Each of these effects may be of particular importance for the optical field induction in the strong coupling regime.…”
Section: Discussionmentioning
confidence: 99%
“…The mechanism of the optical field formation discussed here is related to renormalization of the electron energy spectrum of bulk GaAs in the field of elliptically polarized light wave and to enhancement of the electromagnetic field intensity in microcavities. Besides, semiconductor microcavities demonstrate a variety of specific polarization-dependent linear and nonlinear effects 45 46 47 48 , including polarization conversion, self-induced Larmor precession, second harmonic generation, spin to angular momentum conversion, etc. Each of these effects may be of particular importance for the optical field induction in the strong coupling regime.…”
Section: Discussionmentioning
confidence: 99%
“…A density ordered superfluid is generated to avoid frustration. These on-site pairing terms are natural in Kerr cavity systems [27], exciton-polariton systems [28,29] as well as in NMR systems with antipunching technique [30]. However, the previous work is only focused on the weak interaction region where the density order is generated in presence of any weak pairing term.…”
mentioning
confidence: 99%
“…This provides interesting perspectives for functional polariton circuits and classical polariton simulators [37][38][39][40][41]. Resonant injection of dark excitons via two photon absorption [35,42,43] might provide means to create tailored optical potentials without perturbing relaxation dynamics. Finally, typical pulsed excitation experiments on polariton systems employ lasers with a pulse separation of about 13 ns.…”
mentioning
confidence: 99%