“…is critical for the development of 2D-material-based photonic and optoelectronic devices [ 12 , 13 , 14 , 15 , 16 , 17 ]. Nonlinear saturable absorption is essential for generation of ultrafast laser pulses, which has been widely applied in bulk, fiber, and waveguide laser systems [ 18 , 19 , 20 , 21 , 22 , 23 ]. Recently, the prominent third-order optical nonlinearities and saturable absorption performance of CH 3 NH 3 PbBr 3 have been reported [ 24 , 25 , 26 , 27 , 28 ].…”