Nitrogen-Rich Covalent Organic Polymer for Metal-Free Tandem Catalysis and Postmetalation-Actuated High-Performance Water Oxidation
Nilanjan Seal,
Arun Karmakar,
Partha Pratim Mondal
et al.
Abstract:Development of high-performing catalytic materials for selective and mild chemical transformations through adhering to the principles of sustainability remains a central focus in modern chemistry. Herein, we report the template-free assembly of a thermochemically robust covalent organic polymer (COP: 1) from 2,2′-bipyridine-5,5′-dicarbonyl dichloride and 2,4,6-tris(4aminophenyl)triazine as [2 + 3] structural motifs. The two-dimensional (2D) layered architecture contains carboxamide functionality, delocalized π… Show more
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