Nickel-based Single-Molecule Catalysts with Synergistic Geometric Transition and Magnetic Field-assisted Spin Selection Outperforms RuO2 for Oxygen Evolution
Abstract:Overcoming slow kinetics and high overpotential in electrocatalytic oxygen evolution reaction (OER) requires innovative catalysts and approaches that transcend the scaling relationship between binding energies for intermediates and catalyst surfaces. Inorganic complexes provide unique catalyst designs with customizable geometries, which can help enhance their efficiencies. However, they are unstable and susceptible to oxidation under extreme pH conditions. Immobilizing complexes on substrates creates single-mo… Show more
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