An improved method of U-Pb dating of vein calcite formed during deformation is used to determine the age of folding along the south Coast of England, and determine its cause. Fractures arising from folding of Late Cretaceous Chalk of southern England occurred 34.7±1.7 Ma ago. Underlying Jurassic strata have veins within fractures with ages of 55, 48-42, 39-37, 34-31, and 25 Ma, with 34-31 Ma being the tectonic culmination. Folding was slightly younger than the age of the youngest strata in the overlying Solent Group, suggesting folding terminated basin sedimentation. This age of N-S shortening is inconsistent with attribution from intraplate forces from the mainly younger Alps, but is plausibly a result of the Pyrenean orogen that evolved from 50-28 Ma ago with a late Eocene culmination. A modified methodology for carbonate LA-ICP-MS U-Pb dating is presented that uses measured 232 Th and 208 Pb as a better monitor of common Pb, and it has distinct advantages over existing methods. Initial common lead determined on samples conforms closely to Stacey-Kramers (1975) model compositions, with free regressions giving the most robust dates. The modified method is applicable to structural geology, carbonate diagenesis, and to dating of carbonate relevant to palaeo-environmental and archaeological studies. Supplementary material: Appendices 1, 2, 3, 4 and 5 are available at https://doi.org/xxxx' The landscape of the southern coastal region of England from Dorset to Kent is notable historically and for its place in literature, the arts, natural history and tourism. The coastal morphology arises from differential erosion of tilted and folded strata that form escarpments and dramatic coastal cliffs. Folds have been recognised since publication of William Smith's 1815 map more than 200 years ago, for example in early accounts by Webster (1816),