“…A variety of neuromorphic functions, including high-performance analog resistive switching, [3][4][5][6][7][8]10,13 spike timing-dependent plasticity, 4,7 and second-order memristor characteristics, 7 have been demonstrated in thin-film devices of a-TaO x , in addition to the fact that it has been widely used as a practical material for commercial resistive random access memory (ReRAM). 3,10,28 In amorphous metal oxides, three types of analog switching phenomena have been demonstrated depending on the control parameters: (1) analog set (resistance decrease) controlled by the compliance current (I c ), 1,5,6,13 (2) analog reset (resistance increase) controlled by the maximum applied voltage (V max ), 1,3,4,6,8,13 and (3) analog set and reset by multiple voltage applications (i.e., controlled by the voltage application time). 2,4,7,8 In our measurements, all three types of phenomena were directly demonstrated by C-AFM, and the involved ionic migration was observed in the angstrom scale.…”