Near-Infrared Light and Acid/Base Dual-Regulated Polymerization Utilizing Imidazole-Anion-Fused Perylene Diimides as Photocatalysts

Ti, Qihui; Fang, Liping; Zhao, Weihe; Bai, Libin; Zhao, Hongchi; Ba, Xinwu; Chen, Weiping

doi:10.1021/jacs.3c08503

J. Am. Chem. Soc.

2023

DOI: 10.1021/jacs.3c08503

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Near-Infrared Light and Acid/Base Dual-Regulated Polymerization Utilizing Imidazole-Anion-Fused Perylene Diimides as Photocatalysts

Qihui Ti,

Liping Fang,

Weihe Zhao

et al.

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2024

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Cited by 2 publications

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Photochemical Action Plots Reveal Red‐shifted Wavelength‐dependent Photoproduct Distributions

Carroll,

Pashley‐Johnson,

Frisch

et al. 2024

Chemistry A European J

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Photochemical action plots are a powerful tool for mapping photochemical reaction outcomes wavelength‐by‐wavelength. Typically, they map either the depletion of a reactant or the formation of a specific product as a function of wavelength. Herein, we exploit action plots to simultaneously map the formation of several photochemical products from a single chromophore. We demonstrate that the wavelength‐resolved mapping of two reaction products formed during the irradiation of a chalcone species not only shows wavelength dependence – exhibiting the typical strong red‐shift of the photochemical reactivity compared to the absorbance spectrum of the chromophore – but also a strong wavelength selectivity with remarkably different product distributions resulting from different irradiation wavelengths.

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Photochemical Action Plots Reveal Red‐shifted Wavelength‐dependent Photoproduct Distributions

Carroll,

Pashley‐Johnson,

Frisch

et al. 2024

Chemistry A European J

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Recent advancements in the molecular design of deep-red to near-infrared light-absorbing photocatalysts

Zhong,

Sun

2024

Chem Catalysis

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Near-Infrared Light and Acid/Base Dual-Regulated Polymerization Utilizing Imidazole-Anion-Fused Perylene Diimides as Photocatalysts

Cited by 2 publications

References 74 publications

Photochemical Action Plots Reveal Red‐shifted Wavelength‐dependent Photoproduct Distributions

Photochemical Action Plots Reveal Red‐shifted Wavelength‐dependent Photoproduct Distributions

Recent advancements in the molecular design of deep-red to near-infrared light-absorbing photocatalysts

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