Abstract:A novel class of agents is developed based on the core engineering of open‐shelled organic mixed‐valence (MV) systems, which enable tunable absorption and emission across the near infrared (NIR)‐I to III biowindow (700–1850 nm) by adjusting the number of central nitrogen oxidation sites and the length of the conjugated bridge. Organic mixed ‐valence (MV) systems are synthesized through a one‐step partial chemical oxidation of starburst oligoarylamines, with varying nitrogen oxidation sites and conjugated bridge… Show more
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